Publications

Long distance quantum networking requires combining efficient spin-photon interfaces with long-lived local memories. Group-IV color centers in diamond (SiV–, GeV–, and SnV–) are promising candidates for this application, containing an electronic spin-photon interface and dopant nuclear spin memory. Recent work has demonstrated state-of-the-art performance in spin-photon coupling and spin-spin entanglement. However, coupling between the electron and nuclear spins introduces a phase kickback during optical excitation that limits the utility of the nuclear memory. Here, we propose using the large hyperfine coupling of 117SnV– to operate the device at zero magnetic field in a regime where the memory is insensitive to optical excitation. We further demonstrate ground state spin control of a 117SnV– color center integrated in a photonic integrated circuit, showing 97.8% gate fidelity and 2.5 ms coherence time for the memory spin level. This shows the viability of the zero-field protocol for high fidelity operation, and lays the groundwork for building quantum network nodes with 117SnV– devices.

Solid-state quantum sensors are attracting wide interest because of their sensitivity at room temperature. In particular, the spin properties of individual nitrogen-vacancy (NV) colour centres in diamond make them outstanding nanoscale sensors of magnetic fields, electric fields and temperature under ambient conditions. Recent work on NV ensemble-based magnetometers, inertial sensors, and clocks has employed unentangled colour centres to realize significant improvements in sensitivity. However, to achieve this potential sensitivity enhancement in practice, new techniques are required to excite efficiently and to collect the optical signal from large NV ensembles. Here, we introduce a light-trapping diamond waveguide geometry with an excitation efficiency and signal collection that enables in excess of 5% conversion efficiency of pump photons into optically detected magnetic resonance (ODMR) fluorescence--an improvement over previous single-pass geometries of more than three orders of magnitude. This marked enhancement of the ODMR signal enables precision broadband measurements of magnetic field and temperature in the low-frequency range, otherwise inaccessible by dynamical decoupling techniques.